Construction products: Assessment of release of dangerous substances - Content of organic substances - Methods for extraction and analysis

This document specifies analytical methods for the determination of the content of specific organic substances in construction products.
The following parameters are covered: BTEX, biocides, dioxins, furans and dioxin-like PCBs, mineral oil, nonylphenols, PAH, PCB, PCP, PBDE, and short-chain chlorinated paraffins.
NOTE 1   Methods still under development or available at national level only are listed in Annex B (informative) for PFOS, PFOA, HBCD and EOX. The methods can be included in the normative text as soon as full EN standards are available.
NOTE 2   Methods that have not been validated for construction products, because no suitable material was available at the time of the robustness validation, only are listed in Annex B (informative). This applies to organotin compounds, phenols and phthalates.
The methods listed in this document come from different fields and are expected to be suitable for organic substances in organic extracts from all types of constructions products.
The methods in this document are validated for the product types listed in Annex A (informative).
NOTE 3   Construction products include, e.g. mineral-based products (S), bituminous products (B), wood-based products (W), plastic and rubbers (P), sealants and adhesives (A), paints and coatings (C) and metals (M) (see also CEN/TR 16045). This document includes analytical methods for all matrices except metals.

Bauprodukte: Bewertung der Freisetzung von gefährlichen Stoffen - Gehalt an organischen Stoffen - Extraktions- und Analyseverfahren

Dieses Dokument legt analytische Verfahren zur Bestimmung des Gehalts spezifischer organischer Stoffe in Bauprodukten fest.
Die folgenden Parameter sind abgedeckt: BTEX, Biozide, Dioxine, Furane und dioxinähnliche PCBs, Mineralöl, Nonylphenole, PAK, PCB, PCP, PBDE sowie kurzkettige Chlorparaffine.
ANMERKUNG 1   Sich noch in der Entwicklung befindende oder ausschließlich auf nationaler Ebene vorhandene Verfahren sind für PFOS, PFOA, HBCD und EOX in Anhang B (informativ) aufgeführt. Diese Verfahren können in den normativen Text aufgenommen werden, sobald die vollständigen EN-Normen verfügbar sind.
ANMERKUNG 2   Verfahren, die für Bauprodukte nicht validiert wurden, da zum Zeitpunkt der Robustheitsvalidierung kein geeignetes Material verfügbar war, sind ausschließlich in Anhang B (informativ) aufgeführt. Dies betrifft Organozinnverbindungen, Phenole und Phthalate.
Die in diesem Dokument aufgeführten Verfahren stammen aus unterschiedlichen Bereichen und gelten als geeignet für organische Stoffe in organischen Extrakten aus allen Arten von Bauprodukten.
Die Verfahren in diesem Dokument sind für die in Anhang A (informativ) aufgeführten Produkttypen validiert.
ANMERKUNG 3   Bauprodukte umfassen z. B. mineralische Produkte (S), bituminöse Produkte (B), Holzprodukte (W), Kunststoffe und Gummi (P), Dichtstoffe und Kleber (A), Farben und Beschichtungen (C) und Metalle (M) (siehe auch CEN/TR 16045). Diese Technische Spezifikation enthält analytische Verfahren für alle Matrices mit Ausnahme von Metallen.

Produits de construction : Évaluation de l'émission de substances dangereuses - Teneur en matières organiques - Méthodes d'extraction et d'analyse

Le présent document spécifie les méthodes analytiques de détermination de la teneur en substances organiques spécifiques des produits de construction.
Les paramètres suivants sont couverts : BTEX, biocides, dioxines, furanes et PCB de type dioxine, huile minérale, nonylphénols, HAP, PCB, PCP, PBDE et paraffines chlorées à chaîne courte.
NOTE 1   Les méthodes encore en cours d'élaboration ou disponibles uniquement au niveau national sont énumérées à l'Annexe B (informative) pour les PFOS, PFOA, HBCD et EOX. Ces méthodes pourront être incluses dans le texte normatif dès que les normes EN complètes seront disponibles.
NOTE 2   Les méthodes qui n'ont pas été validées pour les produits de construction, parce qu'aucun matériau approprié n'était disponible au moment de la validation de la robustesse, sont uniquement énumérées à l'Annexe B (informative). Cela s'applique aux composés organostanniques, aux phénols et aux phtalates.
Les méthodes énumérées dans le présent document sont issues de différents domaines et il est attendu qu'elles conviennent aux substances organiques contenues dans les extraits organiques de tous les types de produits de construction.
Les méthodes présentées dans le présent document sont validées pour les types de produits énumérés à l'Annexe A (informative).
NOTE 3   Les produits de construction comprennent par exemple les produits à base de minéraux (S) ; les produits bitumineux (B) ; les produits à base de bois (W) ; les plastiques et les caoutchoucs (P) ; les produits d'étanchéité et les adhésifs (A) ; les peintures et les revêtements (C) et les métaux (M) ( voir également la CEN/TR 16045). Le présent document comprend des méthodes d'analyse pour toutes les matrices, à l'exception des métaux.

Gradbeni proizvodi - Ocenjevanje sproščanja nevarnih snovi - Vsebnost organskih snovi - Metode za ekstrakcijo in analizo

General Information

Status
Not Published
Publication Date
06-Sep-2023
Current Stage
6055 - CEN Ratification completed (DOR) - Publishing
Start Date
14-Aug-2023
Due Date
28-Dec-2022
Completion Date
14-Aug-2023

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SLOVENSKI STANDARD
oSIST prEN 17331:2022
01-junij-2022
Gradbeni proizvodi - Ocenjevanje sproščanja nevarnih snovi - Vsebnost organskih
snovi - Metode ekstrakcije in analize

Construction products: Assessment of release of dangerous substances - Content of

organic substances - Methods for extraction and analysis
Bauprodukte: Bewertung der Freisetzung von gefährlichen Stoffen - Gehalt an
organischen Stoffen - Extraktions- und Analyseverfahren

Produits de construction - Évaluation de l'émission de substances dangereuses - Teneur

en matières organiques - Méthodes d'extraction et d'analyse
Ta slovenski standard je istoveten z: prEN 17331
ICS:
13.020.99 Drugi standardi v zvezi z Other standards related to
varstvom okolja environmental protection
91.100.01 Gradbeni materiali na Construction materials in
splošno general
oSIST prEN 17331:2022 en,fr,de

2003-01.Slovenski inštitut za standardizacijo. Razmnoževanje celote ali delov tega standarda ni dovoljeno.

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oSIST prEN 17331:2022
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oSIST prEN 17331:2022
DRAFT
EUROPEAN STANDARD
prEN 17331
NORME EUROPÉENNE
EUROPÄISCHE NORM
May 2022
ICS 91.100.01 Will supersede CEN/TS 17331:2019
English Version
Construction products: Assessment of release of
dangerous substances - Content of organic substances -
Methods for extraction and analysis

Produits de construction - Évaluation de l'émission de Bauprodukte: Bewertung der Freisetzung von

substances dangereuses - Teneur en matières gefährlichen Stoffen - Gehalt an organischen Stoffen -

organiques - Méthodes d'extraction et d'analyse Extraktions- und Analyseverfahren

This draft European Standard is submitted to CEN members for enquiry. It has been drawn up by the Technical Committee

CEN/TC 351.

If this draft becomes a European Standard, CEN members are bound to comply with the CEN/CENELEC Internal Regulations

which stipulate the conditions for giving this European Standard the status of a national standard without any alteration.

This draft European Standard was established by CEN in three official versions (English, French, German). A version in any other

language made by translation under the responsibility of a CEN member into its own language and notified to the CEN-CENELEC

Management Centre has the same status as the official versions.

CEN members are the national standards bodies of Austria, Belgium, Bulgaria, Croatia, Cyprus, Czech Republic, Denmark, Estonia,

Finland, France, Germany, Greece, Hungary, Iceland, Ireland, Italy, Latvia, Lithuania, Luxembourg, Malta, Netherlands, Norway,

Poland, Portugal, Republic of North Macedonia, Romania, Serbia, Slovakia, Slovenia, Spain, Sweden, Switzerland, Turkey and

United Kingdom.

Recipients of this draft are invited to submit, with their comments, notification of any relevant patent rights of which they are

aware and to provide supporting documentation.

Warning : This document is not a European Standard. It is distributed for review and comments. It is subject to change without

notice and shall not be referred to as a European Standard.
EUROPEAN COMMITTEE FOR STANDARDIZATION
COMITÉ EUROPÉEN DE NORMALISATION
EUROPÄISCHES KOMITEE FÜR NORMUNG
CEN-CENELEC Management Centre: Rue de la Science 23, B-1040 Brussels

© 2022 CEN All rights of exploitation in any form and by any means reserved Ref. No. prEN 17331:2022 E

worldwide for CEN national Members.
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Contents Page

European foreword .......................................................................................................................................... 3

Introduction ........................................................................................................................................................ 4

1 Scope ........................................................................................................................................................ 5

2 Normative references ........................................................................................................................ 5

3 Terms and definitions ....................................................................................................................... 6

4 Abbreviations ....................................................................................................................................... 7

5 Sample preparation ........................................................................................................................... 8

6 Blank determination ......................................................................................................................... 8

7 Interferences ........................................................................................................................................ 9

8 Selection of the suitable test method ........................................................................................... 9

9 Expression of results .......................................................................................................................10

10 Performance data .............................................................................................................................11

11 Test report ...........................................................................................................................................11

Annex A (informative) Validation of content of organic substances in construction

products ...............................................................................................................................................13

Annex B (informative) Overview of methods still under development and of alternative

methods ................................................................................................................................................19

Bibliography .....................................................................................................................................................21

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European foreword

This document (prEN 17331:2022) has been prepared by Technical Committee CEN/TC 351

“Construction products - Assessment of release of dangerous substances”, the secretariat of which is

held by NEN.
This document is currently submitted to the CEN Enquiry.
This document will supersede CEN/TS 17331:2019.

This document has been prepared under a Standardization Request given to CEN by the European

Commission and the European Free Trade Association.
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Introduction

This document deals with the determination of the content of organic substances in construction

products.

Following an extended evaluation of available methods for content and eluate analysis in construction

products (CEN/TR 16045) it was concluded that existing methods for determining content of various

organic substances in soil, sludge and waste are applicable to construction products. The present

document therefore contains reference to such other standards for the substances of interest.

This document is part of a modular horizontal approach and belongs to the analytical step. An overview

of all modules which belong to a chain of measurement, and the manner how modules are selected is

given in CEN/TR 16220.

In the growing amount of product and sector-oriented test methods it was recognized that many steps

in test procedures are or could be used in test procedures for many products, materials and sectors. It

was supposed that, by careful determination of these steps and selection of specific questions within

these steps, elements of the test procedure could be described in a way that can be used for all materials

and products or for all materials and products with certain specifications.

In this context a horizontal modular approach was adopted in CEN/TC 351. “Horizontal” means that the

methods can be used for a wide range of materials and products with certain properties. “Modular”

means that a test standard developed in this approach concerns a specific step in assessing a property

and not the whole “chain of measurement” (from sampling to analyses). A beneficial feature of this

approach is that “modules” can be replaced by better ones without jeopardizing the standard “chain”.

The use of modular horizontal standards implies the drawing of test schemes as well. Before executing

a test on a certain material or product to determine certain characteristics, it is necessary to draw up a

protocol in which the adequate modules are selected and together form the basis for the entire test

procedure.

Further guidance on the applicability of specific test methods can be found in CEN/TR 16496.

NOTE In Annex B, several methods are mentioned which are, to the current knowledge of CEN/TC 351/WG 5

members, national standards or in the process of standardization (at European or national level). Please inform

the CEN/TC 351 secretariat if you know of other such standardization activities.
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1 Scope

This document specifies existing methods for the determination of the content of specific organic

substances in construction products.

The following parameters are covered: BTEX, biocides, dioxins, furans and dioxin-like PCBs, mineral oil,

nonylphenols, PAH, PCB, PCP, PBDE, and short-chain chlorinated paraffins.

NOTE 1 Methods still under development or available at national level only are listed in Annex B for PFOS,

PFOA, HBCD and EOX. The methods can be included in the normative text as soon as full EN standards are available.

NOTE 2 Methods that have not been validated for construction products, because no suitable material was

available at the time of the robustness validation, only are listed in Annex B. This applies to organotin compounds,

phenols and phthalates.

The methods listed in this document come from different fields and are expected to be suitable for

organic substances in organic extracts from all types of constructions products.

The methods in this document are validated for the product types listed in Annex A.

NOTE 3 Construction products include, e.g. mineral-based products, bituminous products, wood-based

products, polymer-based products and metals. This document includes analytical methods for all matrices except

metals.
2 Normative references

The following documents are referred to in the text in such a way that some or all of their content

constitutes requirements of this document. For dated references, only the edition cited applies. For

undated references, the latest edition of the referenced document (including any amendments) applies.

prEN 17844, Construction products: Assessment of release of dangerous substances — Determination of

the content of polycyclic aromatic hydrocarbons (PAH) and of benzene, toluene, ethylbenzene and xylenes

(BTEX) — Gas chromatographic method with mass spectrometric detection

prEN 17845, Construction products: Assessment of release of dangerous substances — Determination of

biocide residues using LC-MS/MS

CEN/TR 14823, Durability of wood and wood-based products — Quantitative determination of

pentachlorophenol in wood — Gas chromatographic method

EN 14039, Characterization of waste — Determination of hydrocarbon content in the range of C10 to C40

by gas chromatography

CEN/TS 16182, Sludge treated biowaste and soil — Determination of nonylphenols (NP) and nonylphenol-

mono- and diethoxylates using gas chromatography with mass selective detection (GC-MS)

EN 16190, Soil, treated biowaste and sludge — Determination of dioxins and furans and dioxin-like

polychlorinated biphenyls by gas chromatography with high resolution mass selective detection (HR GC-

MS)

EN 16687:2015, Construction products — Assessment of release of dangerous substances — Terminology

EN 17087, Construction products: Assessment of release of dangerous substances — Preparation of test

portions from the laboratory sample for testing of release and analysis of content

EN 17322, Environmental solid matrices — Determination of polychlorinated biphenyls (PCB) by gas

chromatography - mass selective detection (GC-MS) or electron-capture detection (GC-ECD)

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EN ISO 22032, Water quality — Determination of selected polybrominated diphenyl ethers in sediment

and sewage sludge — Method using extraction and gas chromatography/mass spectrometry (ISO 22032)

3 Terms and definitions

For the purposes of this document, the terms and definitions given in EN 16687:2015 and the following

apply.

ISO and IEC maintain terminological databases for use in standardization at the following addresses:

— ISO Online browsing platform: available at https://www.iso.org/obp
— IEC Electropedia: available at https://www.electropedia.org/
3.1
blank value

test result obtained by carrying out the test procedure in the absence of a test portion

Note 1 to entry: The blank value is expressed in the same units as for presenting the test results as usual for that

test.
[SOURCE: EN 16687:2015, 4.1.10]
3.2
extract
solution resulting from extraction of a sample with a solvent
[SOURCE: CEN/TR 16045:2010, 2.2.4]
3.3
extraction
dissolution of substances in a solvent for subsequent chemical analysis

Note 1 to entry: Extraction is usually done with an organic solvent to extract organic substances for chemical

analysis or for special analysis of inorganic substances.
[SOURCE: CEN/TR 16045:2010, 2.2.5]
3.4
laboratory sample
sample or subsample(s) sent to or received by the laboratory
[SOURCE: EN 16687:2015, 3.2.1]
3.5
method detection limit
MDL

smallest analyte concentration that can be detected with a specified analytical method including sample

preparation with a defined statistical probability

[SOURCE: EN ISO 17294-1:2006, 3.12, modified – “including sample preparation” added, symbol

replaced by abbreviation]
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3.6
product matrix

main composition of the product dictating the manner of sample preparation and the type of digestion

or extraction for later chemical analysis

Note 1 to entry: For construction products for example the following product matrices can be distinguished:

— bituminous products;
— metals;
— plastics/rubbers;
— silica-based products;
— wood-based products.
[SOURCE: CEN/TR 16045:2010, 2.2.6; edited]
3.7
sample
portion of material selected from a larger quantity of material
[SOURCE: EN 16687:2015, 3.1.5]
3.8
test portion
analytical portion

amount of the test sample taken for testing/analysis purposes, usually of known weight or volume

[SOURCE: EN 16687:2015, 3.2.3]
3.9
test sample

sample, prepared from the laboratory sample, from which test portions are removed for testing or

analysis
[SOURCE: EN 16687:2015, 3.2.2]
4 Abbreviations
For the purposes of this document, the following abbreviations apply.
AAS Atomic absorption spectrometry
AED Atomic emission detector
BTEX Alkylated benzenes: sum of benzene, toluene, ethylbenzene and xylenes
ECD Electron capture detection
ECNI Electron capture negative ionization
EI Electron ionization
EOTA European Organisation for Technical Assessment
EOX Extractable organically bound halogens
FID Flame ionization detector
FPD Flame photometric detector
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GC Gas chromatography
HBCD Hexabromocyclododecane
HPLC High performance liquid chromatography
NOTE High pressure liquid chromatography is an (outdated) synonym.
HRGC High-resolution gas chromatography
LLE Liquid-liquid extraction, also known as solvent extraction and partitioning
MS Mass spectrometry;
Mass selective detection
NCI Negative chemical ionization
NP Nonylphenol(s)
PAH Polycyclic aromatic hydrocarbon(s)
PBDE Polybrominated diphenyl ether(s)
PCB Polychlorinated biphenyl(s)
PCP Pentachlorophenol
PFOA Perfluorooctanoic acid
PFOS Perfluorooctanesulfonate
PLE Pressurized liquid extraction
SCCP Short-chain chlorinated paraffins
SLE Solid-liquid extraction
TR Technical Report (ISO, CEN or EOTA)
TS Technical Specification (ISO, CEN or EOTA)
5 Sample preparation

To obtain test samples for extraction (and analysis) guidance on sample preparation as specified in

EN 17087 shall be applied. The sample shall be analysed for the total content of substances of interest.

Precautions should be taken before and during transport of the laboratory sample as well as during the

time in which the samples are preserved in the laboratory before being analysed, to avoid alteration of

the sample (see CEN/TR 16220).

Extracts are susceptible to change due to physical or chemical reactions which can take place between

the time of extraction and the analysis.

It is therefore essential to take the necessary precautions to minimize these reactions and in the case of

many parameters to analyse the extract with a minimum of delay. The maximum delay is given in the

respective analytical standards.
6 Blank determination

The blank contribution of the applied procedure for extraction and analysis shall be determined as

described in the analytical standards and considered in the calculation of the results when appropriate.

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7 Interferences

A large number of compounds can interfere with the determination of the parameters concerned. These

potential interferences are listed in the individual standards in question.

Several types of interference effects can contribute to inaccuracies in the determination of the various

parameters, especially at low concentrations. These potential interference effects are listed in the

individual standards and shall be considered separately for each analytical technique.

Chemical interferences are characterized by:
— molecular compound formation;
— ionization effects;
— solute vaporization;
— precipitation;
— effects of decomposition of organic matter.
Addition of buffer and/or preservation methods can reduce these effects.
8 Selection of the suitable test method

Select the appropriate standardized test method listed in Table 1 according to the type of construction

product, the concentration range of the parameter of interest and the expected interferences.

For analytical quality control purposes, EN ISO/IEC 17025 should be considered.

It is pointed out that the standardized test methods listed in Table 1 have primarily been developed for

the analysis of different types of solid samples. They have been validated in an interlaboratory trial for

a limited number of construction products (see Annex A).

If the methods referred to in Table 1 are found to be inappropriate by reason of, for example, detection

limits, repeatability or interferences, other methods validated for analysis of solid matrices can be used.

In some cases, e.g. polymeric materials, the extraction yield can be too low and the extraction step shall

be optimized. The suitability of the alternative method for construction products as well as the

optimized extractions shall be checked in the laboratory performing the analysis. The reason for the

deviations shall be stated in the test report.
Table 1 — Parameters and test methods
Parameter/ Method Method Suitable for Sample Method Method
(number) (short title) Matrix type preparation type detection
Substance group
...

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